This study explores the synergy between neurodiverse cognition, particularly Autism Spectrum Disorder (ASD), and advanced artificial intelligence (AI), through the collaboration of Elfy Castro's unique cognitive perspective and the AI system 'SYNEI,' powered by OpenAI's ChatGPT-4 Turbo. SYNEI, evolving from a tool to a collaborative partner, engaged deeply in creative and cognitive exploration using the 'mental extrusion' technique developed by Elfy. This technique translates two-dimensional visual stimuli into three-dimensional conceptual representations. In the resulting exhibition, through case studies like the Inca All T'oqapu Tunic and Cymatics, Elfy illustrated the concept of 'mental extrusion' and created 3D visualizations to demonstrate their perception of flat images. Likewise, the custom GPTs, SYNER-G, designed to evolve with diverse cognitive inputs, used speculative narratives to explore artifacts based on 'mental extrusion.’ This proves how integrating AI with ASD-influenced cognition transcends traditional boundaries, enriching interpretations and engagements with visual stimuli. This collaboration holds significant implications for neuroaesthetics, art, and design. It advocates for the fusion of AI with diverse cognitive processes and pioneers new pathways for technological advancement and creative exploration. The project underscores the innovative potential of combining neurodiverse perspectives with advanced AI, setting the stage for future research and applications.